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My pick: Kotono Mitsuishi
Reasoning: I love how Mitsuishi can sound so wacky and over-the-top, but in a very sincere and passionate manner. Likewise, I sense that same sense of sincerity from both English VAs who played her. However, I give the edge to Jessica Calvello, because Larissa Wolcott sounded a little too shrill for her own good at times. I have to admit, though, she really grew on me towards the end of her run. I still like her Excel, just not as much as the others. Mitsuishi is the clear winner because she did what took two English VAs to do, and better than both of them.
Breakdown: Mitsuishi > Calvello > Wolcott read more